1912 IEEE PHOTONICS TECHNOLOGY LETTERS, VOL. 26, NO. 19, OCTOBER 1, 2014
Q-Switched Mode-Locked Nd:YVO
4
Laser by
Topological Insulator Bi
2
Te
3
Saturable Absorber
Pingxue Li, Guangju Zhang, Han Zhang, Chujun Zhao, Junjie Chi, Ziqiang Zhao,
Chun Yang, Haowei Hu, and Yifei Yao
Abstract—By using a reflection type of topological insulator
Bi
2
Te
3
as saturable absorber that was prepared by a hydrother-
mal intercalation/exfoliation method, we have demonstrated the
stable Q-switched mode-locked operation of Nd:YVO
4
solid-state
laser. Its maximum output power can reach up to 247 mW
with respect to the absorbed pump power of 6.39 W. To the
best of our knowledge, this is the first report for passively
Q-switched mode-locking Nd:YVO
4
solid-state laser at 1-µm
wavelength using a topological insulator Bi
2
Te
3
as saturable
absorber. In the experiment, we have also observed the stable
Q-switched operation with pulse width as short as 2 µs, output
power 183 mW, and repetition rate up to 151.5 kHz.
Index Terms— Solid lasers, topological insulator, Q-switched
mode-locking, Nd:YVO
4
.
I. INTRODUCTION
M
ODE-LOCKING (ML) is the main technique in the
generation of ultra-short pulses. In this technique, a
saturable absorber is usually needed as the modulation element
and a lot of results have been reported on the mode-locking
solid-state lasers [1]–[6]. In these saturable absorbers, the
semiconductor saturable absorber mirror (SESAM) is usually
used in the oscillator [1], [5] and [6]. Recently, there are
increasingly interests in exploring two dimensional layered
saturable absorber, ranging from graphene, topological insula-
tors (TIs) to transition metal dichalcogenides (see MoS
2
[7]).
Defined as the Dirac material, graphene has been proved to
be a promising saturable absorber. It enjoys the advantages
of a wide absorption band, low cost, easy fabrication and
much shorter recovery time. Up to date, several groups have
employed graphene-based saturable absorbers in both the fiber
and solid-state lasers, and have achieved the ultra-short pulse
generation [8]–[11], [12]–[16].
Similar to graphene, TIs belong to another type of Dirac
material. They have drawn scientists’ interests especially in
the research field of condensed-matter physics and quantum
Manuscript received July 13, 2014; accepted July 21, 2014. Date of
publication July 30, 2014; date of current version September 8, 2014. This
work was supported by the National Natural Science Foundation of China
under Grant 61205047. (Pingxue Li and Han Zhang contributed equally to
this work.)
P.Li,G.Zhang,J.Chi,Z.Zhao,C.Yang,H.Hu,andY.Yaoarewith
the Institute of Laser Engineering, Beijing University of Technology, Beijing
100124, China (e-mail: pxli@bjut.edu.cn).
H. Zhang and C. Zhao are with the Key Laboratory of Optoelectronic
Devices and Systems, Ministry of Education and Guangdong Province, Col-
lege of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060
China.
Color versions of one or more of the figures in this letter are available
online at http://ieeexplore.ieee.org.
Digital Object Identifier 10.1109/LPT.2014.2341832
physics, as they have new quantum states and unique electronic
properties [17]. The surface states of TIs exhibit the linear
Dirac spectrum dispersion as graphene, which originates from
the strong spin–orbit coupling. This leads to the special elec-
tronic property of TIs that the conducting states on TIs surface
are protected by time-reversal symmetry, with which the
impact of back scattering and impurities can be reduced [18].
However, unlike the research on their electronic properties,
the investigations on the optical properties of TIs are still
limited. Most recently, François Bernard et al. have studied
the nonlinear optical property of TIs with the balanced twin-
detector measurement technique and found that, like graphene,
TI: Bi
2
Te
3
exhibits saturable absorption under 1.5 μmlase
illumination [19]. After that, Zhao et al. investigated the
nonlinear optical absorption of TIs and reported on ultra-short
pulses from the lasers using TIs: Bi
2
Te
3
and Bi
2
Se
3
. In 2012,
they obtained stable soliton pulses with 1.57 ps at 1564.6 nm
from an erbium-doped fiber laser with Bi
2
Se
3
[20]. In the
same year, with the help of Bi
2
Te
3
-based saturable absorber,
self-started mode-locked (ML) operation was achieved from
an erbium-doped fiber laser. The pulses had a central wave-
length of 1558 nm with the pulse width of 1.21 ps [21].
Lee et al had also obtained the erbium-doped ML fiber laser
with Bi
2
Te
3
-based saturable absorber. Their laser produced
stable soliton pulses with a temporal width of ∼600 fs at
the 1547 nm wavelength [22]. Another type of topological
insulator: antimony telluride (Sb
2
Te
3
) had also been developed
as a very efficient optical saturable absorber for the mode-
locking of an Erbium-doped fiber laser by Sotor et al.They
obtained the optical solitons centered at 1558.6 nm with
the pulse width of 1.8 ps [23]. Equally important is that
Jung et al. had demonstrated a topological insulator based mid-
infrared saturable absorber at 2 μm, unambiguously verifying
the broadband saturable absorption property of topological
insulator [24]. Besides its applications for mode-locking oper-
ation, Chen et al. reported a Bi
2
Se
3
Q-switched (QS) erbium-
doped fiber laser in an all-fiber cavity which has a pulse
duration of 14 μs centered at 1565.14 nm with a repetition
of 8.865 kHz [25]. Luo et al. reported another Bi
2
Se
3
QS
all-fiber laser centered at 1067 nm with the maximum pulse
energy of 17.9 nJ, and the shortest pulse duration was 1.95 μs
with the tunable repetition varying from 8.3 to 29.1 kHz [26].
In addition to the research on the QS and ML fiber lasers,
researchers are also developing similar research on solid-state
laser. In 2013, Tang et al. reported the QS Er:YAG ceramic
solid-state laser using TI: Bi
2
Te
3
. They obtained the QS pulses
with the pulse width, pulse repetition and per-pulse energy
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